I have replaced all the bushes and ball joints in the front suspension. I have set up the castor, camber and toe. This all produced a massive improvement in the feel of the car.
When you drive straight on a smooth road or are settled into a corner, it is fine. Transitioning between the two states is when it feels unsettled (or unsettling!).
I think it comes from the power steering valve/steering box design. If you hit a pothole the wheel gets deflected and then the power steering reacts to correct it, combining the movement in the PAS system with clearances in the steering box, gives a feeling of lack of control. The reality is probably that the car doesn’t deviate much but it doesn’t inspire confidence, likewise when you are changing direction rapidly. I am hoping that the rack will remove that feeling.